Picture: Freddie eats a biscuit while studying at Ealing Technical College in London in summer 1969.
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Watch: Images include relaxing in Prince Hotel, Tokyo when the band were on their Japanese tour there in 1975 - and would go on to tour there another five times - to the frontman leaving the helicopter at the famous Knebworth concert in 1986.
The pair met in 1969 when Mary was just 19-years-old and Freddie was 24.
Footage on the documentary is of one of Freddie most famous solo interviews at Musicland Studios, in Munich, 1984, in which the star.